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Preparation of Bio-hydrogen and Bio-fuels from Lignocellulosic Biomass Pyrolysis-Oil
Pei-wen Jiang,Xiao-ping Wu,Jun-xu Liu,Quan-xin Li
Author NameAffiliationE-mail
Pei-wen Jiang Department of Chemical Physics, Anhui Key Laboratory of Biomass Clean Energy, Key Laboratory of Urban Pollutant Conversion, Chinese Academy of Sciences, University of Science and Technology of China, Hefei 230026, China  
Xiao-ping Wu Department of Chemical Physics, Anhui Key Laboratory of Biomass Clean Energy, Key Laboratory of Urban Pollutant Conversion, Chinese Academy of Sciences, University of Science and Technology of China, Hefei 230026, China  
Jun-xu Liu Department of Chemical Physics, Anhui Key Laboratory of Biomass Clean Energy, Key Laboratory of Urban Pollutant Conversion, Chinese Academy of Sciences, University of Science and Technology of China, Hefei 230026, China  
Quan-xin Li Department of Chemical Physics, Anhui Key Laboratory of Biomass Clean Energy, Key Laboratory of Urban Pollutant Conversion, Chinese Academy of Sciences, University of Science and Technology of China, Hefei 230026, China liqx@ustc.edu.cn 
Abstract:
In recent years, production of engine fuels and energy from biomass has drawn much interest. In this work, we conducted a novel integrated process for the preparation of bio-hydrogen and bio-fuels using lignocellulosic biomass pyrolysis-oil (bio-oil). The process includes (i) the production of bio-hydrogen or bio-syngas by the catalytic cracking of bio-oil, (ii) the adjustment of bio-syngas, and (iii) the production of bio-fuels by ole nic polymerization (OP) together with Fischer-Tropsch synthesis (FTS). Under the optimal conditions, the yield of bio-hydrogen was 120.9 g H2/(kg bio-oil). The yield of hydrocarbon bio-fuels reached 526.1 g/(kg bio-syngas) by the coupling of OP and FTS. The main reaction pathways (or chemical processes) were discussed based on the products observed and the catalyst property.
Key words:  Biomass pyrolysis-oil  Bio-hydrogen  Ole ns polymerization  Fischer-Tropsch synthesis  Bio-fuels
FundProject:
生物油制备生物质氢气和生物质燃料
姜沛汶,吴小平,刘俊旭,李全新
摘要:
研究了一种以生物质裂解油为原料制备氢气和生物燃料的催化转化过程。该过程包括生物油催化裂解制备氢气和生物合成气,合成气的调变,烯烃聚合和费脱合成耦合制备生物燃料。在优化反应条件下,氢气产率达到120.9 g H2/(kg bio-oil),烯烃聚合-费脱合成耦合反应形成的生物燃料产率达到526.1 g/(kg bio-syngas)。基于产物分析和催化剂特性表征,探讨了生物燃料合成过程中的反应路径和化学反应过程.
关键词:  生物油  生物质氢气  烯烃聚合  费脱合成  生物燃料
DOI:10.1063/1674-0068/29/cjcp1603056
分类号: