Xian-ting Liang. Long-Lived Coherence Originating from Electronic-Vibrational Couplings in Light-Harvesting Complexes[J]. Chinese Journal of Chemical Physics , 2017, 30(2): 186-192. doi: 10.1063/1674-0068/30/cjcp1609188
Citation: Xian-ting Liang. Long-Lived Coherence Originating from Electronic-Vibrational Couplings in Light-Harvesting Complexes[J]. Chinese Journal of Chemical Physics , 2017, 30(2): 186-192. doi: 10.1063/1674-0068/30/cjcp1609188

Long-Lived Coherence Originating from Electronic-Vibrational Couplings in Light-Harvesting Complexes

doi: 10.1063/1674-0068/30/cjcp1609188
  • Received Date: 2016-09-25
  • Rev Recd Date: 2016-11-14
  • We theoretically investigate the evolutions of two-dimensional, third-order, nonlinear pho-ton echo rephasing spectra with population time by using an exact numerical path integral method. It is shown that for the same system, the coherence time and relaxation time of excitonic states are short, however, if the couplings of electronic and intra-pigment vibra-tional modes are considered, the coherence time and relaxation time of this vibronic states are greatly extended. It means that the couplings between electronic and vibrational modes play important roles in keeping long-lived coherence in light-harvesting complexes. Particularly, by using the method we can fix the transition path of the energy transfer in bio-molecular systems.

     

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