飞秒泵浦-探测实验数据分析
Data Analysis for Pump-probe Experiment with Femtosecond Pulses
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摘要: 陈述了几种获取飞秒泵浦-探测实验数据中的光解动力学信息的解析物理模型.其中单分量和双分量模型用来解释母体分子的单通道和双通道解离过程,另一个单分量模型用来解释碎片分子的解离或去激发过程.所有模型都结合泵浦-探测实验数据予以解释.Abstract: Various analytical physical models are presented to extract the photodissociation dynamics information from the data obtained in the femtosecond pump-probe experiment. The single- and double-component models are employed to explain the single- and double-channel dissociation of parent molecules. Another single-component model for fragment dissociation or deexcitation is also presented. All cases are explanatorily demonstrated on the pump-probe experimental data.