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Danfeng Lou, Rui Zhang, Yuehui Luo, Quanxin Li. Selective Preparation of Light Olefins from Cellulose-Derived Fermentation Intermediates[J]. Chinese Journal of Chemical Physics . doi: 10.1063/1674-0068/cjcp2301007
Citation: Danfeng Lou, Rui Zhang, Yuehui Luo, Quanxin Li. Selective Preparation of Light Olefins from Cellulose-Derived Fermentation Intermediates[J]. Chinese Journal of Chemical Physics . doi: 10.1063/1674-0068/cjcp2301007

Selective Preparation of Light Olefins from Cellulose-Derived Fermentation Intermediates

doi: 10.1063/1674-0068/cjcp2301007
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  • Corresponding author: E-mail: liqx@ustc.edu.cn
  • Received Date: 2023-01-17
  • Accepted Date: 2023-03-20
  • Available Online: 2023-03-22
  • Directional synthesis of bio-based light olefins has great significance for promoting sustainable development of chemical industry. Present work proves that light olefins can be selectively prepared from the cellulose-derived acetone-butanol-ethanol. This transformation has been achieved by coupling cellulose fermentation and acetone-butanol-ethanol catalytic dehydration over the Ce@SAPO-34 catalyst. The active sites and reusability of the catalyst were investigated. High acetone-butanol-ethanol conversion (91.9%) and high olefin selectivity (86.1%) are achieved. Based on the study of the individual components in acetone-butanol-ethanol, the reaction pathways are put forward.

     

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