Energy Transfer Dynamics between Carbon Quantum Dots and Molybdenum Disulfide Revealed by Transient Absorption Spectroscopy

Ruixiang Wu; Xin Liu; Xiaoshuai Wang; Jingjing Luo; Bin Li; Shengzhi Wang; Xiangyang Miao

doi:10.1063/1674-0068/cjcp2208129

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Ruixiang Wu, Xin Liu, Xiaoshuai Wang, Jingjing Luo, Bin Li, Shengzhi Wang, Xiangyang Miao. Energy Transfer Dynamics between Carbon Quantum Dots and Molybdenum Disulfide Revealed by Transient Absorption Spectroscopy[J]. Chinese Journal of Chemical Physics . doi: 10.1063/1674-0068/cjcp2208129

Citation:

Ruixiang Wu, Xin Liu, Xiaoshuai Wang, Jingjing Luo, Bin Li, Shengzhi Wang, Xiangyang Miao. Energy Transfer Dynamics between Carbon Quantum Dots and Molybdenum Disulfide Revealed by Transient Absorption Spectroscopy[J]. Chinese Journal of Chemical Physics . doi: 10.1063/1674-0068/cjcp2208129

Citation:

Ruixiang Wu, Xin Liu, Xiaoshuai Wang, Jingjing Luo, Bin Li, Shengzhi Wang, Xiangyang Miao. Energy Transfer Dynamics between Carbon Quantum Dots and Molybdenum Disulfide Revealed by Transient Absorption Spectroscopy[J]. Chinese Journal of Chemical Physics . doi: 10.1063/1674-0068/cjcp2208129

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Energy Transfer Dynamics between Carbon Quantum Dots and Molybdenum Disulfide Revealed by Transient Absorption Spectroscopy

doi: 10.1063/1674-0068/cjcp2208129

Key Laboratory of Spectral Measurement and Analysis of Shanxi Province, College of Physics and Information Engineering, Shanxi Normal University, Taiyuan 030031, China

More Information

Corresponding author: E-mail: wuruixiang@sxnu.edu.cn; xymiao@sxnu.edu.cn
Received Date: 2022-08-27
Accepted Date: 2022-09-30

Available Online: 2022-10-01

Abstract

Abstract

Zero-dimensional environmentally friendly carbon quantum dots (CQDs) combined with two-dimensional materials have a wide range of applications in optoelectronic devices. We combined steady-state and transient absorption spectroscopies to study the energy transfer dynamics between CQDs and molybdenum disulfide (MoS₂). Transient absorption plots showed photoinduced absorption and stimulated emission features, which involved the intrinsic and defect states of CQDs. Adding MoS₂ to CQDs solution, the lowest unoccupied molecular orbital of CQDs transferred energy to MoS₂, which quenched the intrinsic emission at 390 nm. With addition of MoS₂,CQDs-MoS₂ composites quenched defect emission at 490 nm and upward absorption, which originated from another energy transfer from the defect state. Two energy transfer paths between CQDs and MoS₂ were efficiently manipulated by changing the concentration of MoS₂, which laid a foundation for improving device performance.
- Energy transfer,
- Transient absorption spectroscopy,
- Carbon quantum dot,
- Molybdenum disulfide

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References(41)

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