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Dec.  2021
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Guo-dong Wang, Zhi-xing Liu, Bei-bei Qiu, Zhi-guo Zhang, Rui Wang, Xiao-yong Wang, Jing Ma, Yong-fang Li, Min Xiao, Chun-feng Zhang. Ultrafast Electron Transfer in All-Small-Molecule Photovoltaic Blends Promoted by Intermolecular Interactions in Cyanided Donors[J]. Chinese Journal of Chemical Physics , 2021, 34(6): 751-760. DOI: 10.1063/1674-0068/cjcp2109179
Citation: Guo-dong Wang, Zhi-xing Liu, Bei-bei Qiu, Zhi-guo Zhang, Rui Wang, Xiao-yong Wang, Jing Ma, Yong-fang Li, Min Xiao, Chun-feng Zhang. Ultrafast Electron Transfer in All-Small-Molecule Photovoltaic Blends Promoted by Intermolecular Interactions in Cyanided Donors[J]. Chinese Journal of Chemical Physics , 2021, 34(6): 751-760. DOI: 10.1063/1674-0068/cjcp2109179
shu

Ultrafast Electron Transfer in All-Small-Molecule Photovoltaic Blends Promoted by Intermolecular Interactions in Cyanided Donors

  • a.

    National Laboratory of Solid State Microstructures, School of Physics, and Collaborative Innovation Center for Advanced Microstructures, Nanjing University, Nanjing 210093, China

  • b.

    Beijing National Laboratory for Molecular Sciences, CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China

  • c.

    State key Laboratory of Chemical Resource Engineering, College of Materials Science and Engineering, Beijing University of Chemical Technology, Beijing 100029, China

  • d.

    Institute of Theoretical and Computational Chemistry, Key Laboratory of Mesoscopic Chemistry of Ministry of Education, School of Chemistry and Chemical Engineering, Nanjing University, Nanjing 210093, China

  • e.

    Department of Physics, University of Arkansas, Fayetteville, Arkansas 72701, USA

More Information
  • Corresponding author:

    Chun-feng Zhang, E-mail: cfzhang@nju.edu.cn

  • Received Date: September 29, 2021
  • Accepted Date: October 11, 2021
  • Available Online: October 18, 2021
  • Issue Publish Date: December 26, 2021
    Graphical Abstract
    • Abstract
  • Cyano substitution has been established as a viable approach to optimize the performance of all-small-molecule organic solar cells. However, the effect of cyano substitution on the dynamics of photo-charge generation remains largely unexplored. Here, we report an ultrafast spectroscopic study showing that electron transfer is markedly promoted by enhanced intermolecular charge-transfer interaction in all-small-molecule blends with cyanided donors. The delocalized excitations, arising from intermolecular interaction in the moiety of cyano-substituted donor, undergo ultrafast electron transfer with a lifetime of ∼3 ps in the blend. In contrast, some locally excited states, surviving in the film of donor without cyano substitution, are not actively involved in the charge separation. These findings well explain the performance improvement of devices with cyanided donors, suggesting that manipulating intermolecular interaction is an efficient strategy for device optimization.
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  • †Part of Special Issue "John Z.H. Zhang Festschrift for celebrating his 60th birthday".

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