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Volume 30 Issue 2
Apr.  2017
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Yan Zhou, Li-qiang Yan, Zhi-neng Kong, Wen-qi Du, Bao-ying Wu, Zheng-jian Qi. Two Rhodamine-based Turn on Chemosensors with High Sensitivity, Selectivity, and Naked-Eye Detection for Hg2+[J]. Chinese Journal of Chemical Physics , 2017, 30(2): 225-230. DOI: 10.1063/1674-0068/30/cjcp1608153
Citation: Yan Zhou, Li-qiang Yan, Zhi-neng Kong, Wen-qi Du, Bao-ying Wu, Zheng-jian Qi. Two Rhodamine-based Turn on Chemosensors with High Sensitivity, Selectivity, and Naked-Eye Detection for Hg2+[J]. Chinese Journal of Chemical Physics , 2017, 30(2): 225-230. DOI: 10.1063/1674-0068/30/cjcp1608153
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Two Rhodamine-based Turn on Chemosensors with High Sensitivity, Selectivity, and Naked-Eye Detection for Hg2+

  • College of Chemistry and Chemical Engineering, Southeast University, Nanjing 211189, China

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  • Received Date: August 04, 2016
  • Revised Date: September 12, 2016
    Graphical Abstract
    • Abstract
  • Two novel rhodamine-based fluorescence enhanced molecular probes (RA1 and RA2) were synthesized, which were both designed as comparative fluoroionophore and chromophore for the optical detection of Hg2+. The recognizing behaviors were investigated both experimentally and computationally. They exhibited high selectivity and sensitivity for Hg2+ over other commonly coexistent metal ions in CH3CN/H2O (1:1, V/V) solution. Test shows that hydroxy benzene of rich electron was beneficial to the chelate of Hg2+ with sensors. The detection limit was measured to be at least 0.14 μmol/L. After addition of Hg2+, the color changed from colourless to pink, which was easily detected by the naked eye in both solution and hydrogel sensor.
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    2. Yan, L., Gu, X., Wang, Z. et al. Fe3+-Responsive Micelle Based on an Amphiphilic Polymer and a Rhodamine B-Containing Amphiphile in Aqueous Media. ChemistrySelect, 2018, 3(12): 3406-3410. DOI:10.1002/slct.201800311
    3. Sakthivel, P., Sekar, K., Sivaraman, G. et al. Rhodamine-benzothiazole conjugate as an efficient multimodal sensor for Hg2+ ions and its application to imaging in living cells. New Journal of Chemistry, 2018, 42(14): 11665-11672. DOI:10.1039/c8nj01736k

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